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Wiedemann-Franz Law
for Magnon Transport
Based on [Phys. Rev. B 92, 134425 (2015)] by KN, P. Simon, and D. Loss
Kouki Nakata
Univ. of Basel
All the responsibility of this slide rests with “Kouki Nakata”
 MAIN MESSAGE
162 YEARS AGO
due to electron (Fermion)
[R. Franz and G. Wiedemann, Annalen der Physik 165, 497 (1853)]
 「Wiedemann-Franz Law」
𝜋2
3
𝑘B
𝑒
2
𝑇
Thermoelectric Effects in Metal
THEN
Thermomagnetic Effects in FI
QUESTION
 How expressed in `AN EQUATION’ ?
due to magnon (Boson)
Universality
𝑘B
𝑔𝜇B
2
𝑇
ANSWER
[KN, P. Simon, and D. Loss, Phys. Rev. B 92, 134425 (2015)]
WHY? We discuss from now on
 BACKGROUND
Universal Thermomagnetic Relation
of Magnon Transport
GOAL
 FI:Long-ranged magnetic order  ``Magnon (spin-wave)’’
𝑘B
𝜇B
Magnet Heat
?
Universal Thermomagnetic Relation
of Magnon Transport
 Thermoelectric properties
of Electron transport in metal
 Wiedemann-Franz Law
Guiding principle
 FI:Long-ranged magnetic order  ``Magnon (spin-wave)’’
GOAL
Wiedemann-Franz Law[R. Franz and G. Wiedemann, Annalen der Physik 165, 497 (1853)]
 Thermoelectric properties of electron transport
Lorenz number ℒ ≡
𝜋2
3
𝑘 𝐵
𝑒
2
: Universal
𝐾
𝜎
=
𝜋2
3
𝑘 𝐵
𝑒
2
𝑇
(𝐾: Thermal conductivity, 𝜎: Electrical conductivity)
Low
temp.
𝑗𝑒
𝑗 𝑄
= 𝐿11
𝐿12
𝐿21
𝐿22
𝐸
𝛻𝑇
charge
Heat
Onsager matrix 𝐿𝑖𝑗
Thermoelectric Effects
Electron (metal) Magnon (FI)
WF law
(Low temp.)
𝐿22
+ 𝑂(𝜀 𝐹
−2
)
𝐿11 ≈
𝐾
𝜎
=
𝜋2
3
𝑘 𝐵
𝑒
2
𝑇 ?
Lorenz
number ℒ ≡
𝜋2
3
𝑘 𝐵
𝑒
2
?
Seebeck 𝑆 &
Peltier Π
𝑆 ≡ 𝐿12
/𝐿11
, 𝛱 ≡ 𝐿21
/𝐿11
Thomson relation: 𝛱 = 𝑇𝑆 ?
Electron (metal) Magnon (FI)
WF law
(Low temp.)
𝐿22
+ 𝑂(𝜀 𝐹
−2
)
𝐿11 ≈
𝐾
𝜎
=
𝜋2
3
𝑘 𝐵
𝑒
2
𝑇 ?
Lorenz
number ℒ ≡
𝜋2
3
𝑘 𝐵
𝑒
2
?
Seebeck 𝑆 &
Peltier Π
𝑆 ≡ 𝐿12
/𝐿11
, 𝛱 ≡ 𝐿21
/𝐿11
Thomson relation: 𝛱 = 𝑇𝑆 ?
𝐼m
𝐼 𝑄
= 𝐿11
𝐿12
𝐿21
𝐿22
𝛻𝐵
𝛻𝑇
Magnet
Heat
Onsager matrix 𝐿𝑖𝑗
Thermomagnetic Effects
𝐼m
𝐼 𝑄
= 𝐿11
𝐿12
𝐿21
𝐿22
𝛻𝐵
𝛻𝑇
WF
Magnet
Heat
Thermomagnetic Effects
Onsager matrix 𝐿𝑖𝑗
Electron (metal) Magnon (FI)
WF law
(Low temp.)
𝐿22
+ 𝑂(𝜀 𝐹
−2
)
𝐿11 ≈
𝐾
𝜎
=
𝜋2
3
𝑘 𝐵
𝑒
2
𝑇
𝐾
𝐺
≡
𝐿22 − 𝐿21 𝐿12/𝐿11
𝐿11
= ?
Lorenz
number ℒ ≡
𝜋2
3
𝑘 𝐵
𝑒
2
ℒm = ?
Seebeck 𝑆 &
Peltier Π
𝑆 ≡ 𝐿12
/𝐿11
, 𝛱 ≡ 𝐿21
/𝐿11
Thomson relation: 𝛱 = 𝑇𝑆
What is their behaviors at low temp. ?
Charge
𝑒
Magnet
𝜇B
Heat
𝑘B
TARGET
Fermion VS Boson
``Wiedemann-Franz Law’’
[R. Franz and G. Wiedemann, Annalen der Physik 165, 497 (1853)]
[KN, P. Simon, and D. Loss, Phys. Rev. B 92, 134425 (2015)]
Point
 Thermal properties “𝒌 𝐁”:Different ? OR Universal ?
Magnon Wiedemann-Franz Law
 Quantum-statistical properties are different
Electron 𝒆 = Fermion
Magnon 𝜇B = Boson
 SYSTEM
[KN, P. Simon, and D. Loss, Phys. Rev. B 92, 134425 (2015)]
Ferromagnetic Insulating Junction
 𝐽ex ≪ 𝐽
(weak coupling)
𝑇L
𝑇R
∆𝐵 ≡ 𝐵R − 𝐵L
∆𝑇 ≡ 𝑇R − 𝑇L
Magnon currents
Q. What happen when magnons are in condensation ?
 See [PRB 90, 144419 (2014)] & [PRB 92, 014422 (2015)]
Onsager matrix 𝐿𝑖𝑗
Magnetic current
Heat current
𝐽ex ≪ 𝐽,
( 𝑎: Lattice constant)
∆𝐵 ≡ 𝐵R − 𝐵L, ∆𝑇 ≡ 𝑇R − 𝑇L
𝑇R
𝑇L
Ferromagnetic Insulating Junction
𝐿11
∝ 𝜇B
2
𝐿22
∝ 𝑘B
2
𝐿12
∝ 𝜇B 𝑘B
𝐿21
∝ 𝜇B 𝑘B
 RESULTS
[KN, P. Simon, and D. Loss, Phys. Rev. B 92, 134425 (2015)]
 Magnon Lorenz number: ℒm ≡
𝑘 𝐵
𝑔𝜇 𝐵
2
: `Universal’
𝐾
𝐺
=
𝑘 𝐵
𝑔𝜇 𝐵
2
𝑇 ∝ 𝑇
 Thermal magnon conductance: 𝐾 ≡ 𝐿22 − 𝐿21 𝐿12/𝐿11
 Magnetic magnon conductance: 𝐺 ≡ 𝐿11
Thermomagnetic Effects
Low temp.: ℏ/(2𝜏) ≪ 𝑘 𝐵 𝑇 ≪ 𝑔𝜇 𝐵 𝐵
Wiedemann-Franz Law for Magnon
(𝜏:Magnon lifetime)
Magnon
(Boson)
Electron
(Fermion)
`Universal’
e vs 𝝁 𝑩 Electron (metal) Magnon (FI)
R. Franz and G. Wiedemann
[Annalen der Physik 165, 497 (1853)]
KN, P. Simon, and DL
[Phys. Rev. B 92, 134425 (2015)]
Fermion Boson
WF law
(Low temp.)
𝐿22
+ 𝑂(𝜀 𝐹
−2
)
𝐿11
≡
𝐾
𝜎
=
𝜋2
3
𝑘 𝐵
𝑒
2
𝑇
(Free electron at low temp.)
𝐿22
− 𝐿21
𝐿12
/𝐿11
𝐿11
≡
𝐾
𝐺
=
𝑘 𝐵
𝑔𝜇 𝐵
2
𝑇
[Low temp.: ℏ/(2𝜏) ≪ 𝑘 𝐵 𝑇 ≪ 𝑔𝜇 𝐵 𝐵]
Lorenz
number ℒ ≡
𝜋2
3
𝑘 𝐵
𝒆
2
ℒm ≡
𝑘 𝐵
𝒈𝝁 𝑩
2
Seebeck 𝑆 &
Peltier Π
𝑆 ≡ 𝐿12
/𝐿11
, 𝛱 ≡ 𝐿21
/𝐿11 𝑆 = 𝐵/𝑇, 𝛱 = 𝐵
[Low temp.: ℏ/(2𝜏) ≪ 𝑘 𝐵 𝑇 ≪ 𝑔𝜇 𝐵 𝐵]
 Universal
Onsager
relation
𝐿21
= 𝑇𝐿12
𝐿21
= 𝑇𝐿12
Thomson
relation
𝛱 = 𝑇𝑆 𝛱 = 𝑇𝑆
Thermo-electric & –magnetic Effects
CONCLUSION
Ratio of 𝐿𝑖𝑗
: 𝐾/𝐺, 𝑆, 𝛱
 Universal thermomagnetic properties
(i.e., Not depend on materials)
 Each Onsager coefficient 𝐿𝑖𝑗: Depend on materials
SUMMARY
𝐾
𝐺
=
𝑘 𝐵
𝑔𝜇 𝐵
2
𝑇 ∝ 𝑇
𝐾 : Thermal magnon conductance, 𝐺: Magnetic magnon conductance
Wiedemann-Franz Law for Magnon
 Fundamental thermomagnetic relation of magnon transport in FI
 Ratio of 𝐿𝑖𝑗: 𝐾/𝐺, 𝑆, 𝛱  Universal thermomagnetic properties
Low temp.: ℏ/(2𝜏) ≪ 𝑘 𝐵 𝑇 ≪ 𝑔𝜇 𝐵 𝐵
𝑘B𝜇B `WF’
Magnet: 𝐺 Heat: 𝐾
Magnon
(Boson)
Electron
(Fermion)
`Universal’
Based on [Phys. Rev. B 92, 134425 (2015)] by KN, P. Simon, and D. Loss

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Wiedemann-Franz Law for Magnon Transport

  • 1. Wiedemann-Franz Law for Magnon Transport Based on [Phys. Rev. B 92, 134425 (2015)] by KN, P. Simon, and D. Loss Kouki Nakata Univ. of Basel All the responsibility of this slide rests with “Kouki Nakata”
  • 3. 162 YEARS AGO due to electron (Fermion) [R. Franz and G. Wiedemann, Annalen der Physik 165, 497 (1853)]  「Wiedemann-Franz Law」 𝜋2 3 𝑘B 𝑒 2 𝑇 Thermoelectric Effects in Metal
  • 5. Thermomagnetic Effects in FI QUESTION  How expressed in `AN EQUATION’ ? due to magnon (Boson) Universality
  • 6. 𝑘B 𝑔𝜇B 2 𝑇 ANSWER [KN, P. Simon, and D. Loss, Phys. Rev. B 92, 134425 (2015)]
  • 7. WHY? We discuss from now on
  • 9. Universal Thermomagnetic Relation of Magnon Transport GOAL  FI:Long-ranged magnetic order  ``Magnon (spin-wave)’’ 𝑘B 𝜇B Magnet Heat ?
  • 10. Universal Thermomagnetic Relation of Magnon Transport  Thermoelectric properties of Electron transport in metal  Wiedemann-Franz Law Guiding principle  FI:Long-ranged magnetic order  ``Magnon (spin-wave)’’ GOAL
  • 11. Wiedemann-Franz Law[R. Franz and G. Wiedemann, Annalen der Physik 165, 497 (1853)]  Thermoelectric properties of electron transport Lorenz number ℒ ≡ 𝜋2 3 𝑘 𝐵 𝑒 2 : Universal 𝐾 𝜎 = 𝜋2 3 𝑘 𝐵 𝑒 2 𝑇 (𝐾: Thermal conductivity, 𝜎: Electrical conductivity) Low temp.
  • 12. 𝑗𝑒 𝑗 𝑄 = 𝐿11 𝐿12 𝐿21 𝐿22 𝐸 𝛻𝑇 charge Heat Onsager matrix 𝐿𝑖𝑗 Thermoelectric Effects Electron (metal) Magnon (FI) WF law (Low temp.) 𝐿22 + 𝑂(𝜀 𝐹 −2 ) 𝐿11 ≈ 𝐾 𝜎 = 𝜋2 3 𝑘 𝐵 𝑒 2 𝑇 ? Lorenz number ℒ ≡ 𝜋2 3 𝑘 𝐵 𝑒 2 ? Seebeck 𝑆 & Peltier Π 𝑆 ≡ 𝐿12 /𝐿11 , 𝛱 ≡ 𝐿21 /𝐿11 Thomson relation: 𝛱 = 𝑇𝑆 ?
  • 13. Electron (metal) Magnon (FI) WF law (Low temp.) 𝐿22 + 𝑂(𝜀 𝐹 −2 ) 𝐿11 ≈ 𝐾 𝜎 = 𝜋2 3 𝑘 𝐵 𝑒 2 𝑇 ? Lorenz number ℒ ≡ 𝜋2 3 𝑘 𝐵 𝑒 2 ? Seebeck 𝑆 & Peltier Π 𝑆 ≡ 𝐿12 /𝐿11 , 𝛱 ≡ 𝐿21 /𝐿11 Thomson relation: 𝛱 = 𝑇𝑆 ? 𝐼m 𝐼 𝑄 = 𝐿11 𝐿12 𝐿21 𝐿22 𝛻𝐵 𝛻𝑇 Magnet Heat Onsager matrix 𝐿𝑖𝑗 Thermomagnetic Effects
  • 14. 𝐼m 𝐼 𝑄 = 𝐿11 𝐿12 𝐿21 𝐿22 𝛻𝐵 𝛻𝑇 WF Magnet Heat Thermomagnetic Effects Onsager matrix 𝐿𝑖𝑗 Electron (metal) Magnon (FI) WF law (Low temp.) 𝐿22 + 𝑂(𝜀 𝐹 −2 ) 𝐿11 ≈ 𝐾 𝜎 = 𝜋2 3 𝑘 𝐵 𝑒 2 𝑇 𝐾 𝐺 ≡ 𝐿22 − 𝐿21 𝐿12/𝐿11 𝐿11 = ? Lorenz number ℒ ≡ 𝜋2 3 𝑘 𝐵 𝑒 2 ℒm = ? Seebeck 𝑆 & Peltier Π 𝑆 ≡ 𝐿12 /𝐿11 , 𝛱 ≡ 𝐿21 /𝐿11 Thomson relation: 𝛱 = 𝑇𝑆 What is their behaviors at low temp. ?
  • 15. Charge 𝑒 Magnet 𝜇B Heat 𝑘B TARGET Fermion VS Boson ``Wiedemann-Franz Law’’ [R. Franz and G. Wiedemann, Annalen der Physik 165, 497 (1853)] [KN, P. Simon, and D. Loss, Phys. Rev. B 92, 134425 (2015)]
  • 16. Point  Thermal properties “𝒌 𝐁”:Different ? OR Universal ? Magnon Wiedemann-Franz Law  Quantum-statistical properties are different Electron 𝒆 = Fermion Magnon 𝜇B = Boson
  • 17.  SYSTEM [KN, P. Simon, and D. Loss, Phys. Rev. B 92, 134425 (2015)]
  • 18. Ferromagnetic Insulating Junction  𝐽ex ≪ 𝐽 (weak coupling) 𝑇L 𝑇R ∆𝐵 ≡ 𝐵R − 𝐵L ∆𝑇 ≡ 𝑇R − 𝑇L Magnon currents Q. What happen when magnons are in condensation ?  See [PRB 90, 144419 (2014)] & [PRB 92, 014422 (2015)]
  • 19. Onsager matrix 𝐿𝑖𝑗 Magnetic current Heat current 𝐽ex ≪ 𝐽, ( 𝑎: Lattice constant) ∆𝐵 ≡ 𝐵R − 𝐵L, ∆𝑇 ≡ 𝑇R − 𝑇L 𝑇R 𝑇L Ferromagnetic Insulating Junction 𝐿11 ∝ 𝜇B 2 𝐿22 ∝ 𝑘B 2 𝐿12 ∝ 𝜇B 𝑘B 𝐿21 ∝ 𝜇B 𝑘B
  • 20.  RESULTS [KN, P. Simon, and D. Loss, Phys. Rev. B 92, 134425 (2015)]
  • 21.  Magnon Lorenz number: ℒm ≡ 𝑘 𝐵 𝑔𝜇 𝐵 2 : `Universal’ 𝐾 𝐺 = 𝑘 𝐵 𝑔𝜇 𝐵 2 𝑇 ∝ 𝑇  Thermal magnon conductance: 𝐾 ≡ 𝐿22 − 𝐿21 𝐿12/𝐿11  Magnetic magnon conductance: 𝐺 ≡ 𝐿11 Thermomagnetic Effects Low temp.: ℏ/(2𝜏) ≪ 𝑘 𝐵 𝑇 ≪ 𝑔𝜇 𝐵 𝐵 Wiedemann-Franz Law for Magnon (𝜏:Magnon lifetime) Magnon (Boson) Electron (Fermion) `Universal’
  • 22. e vs 𝝁 𝑩 Electron (metal) Magnon (FI) R. Franz and G. Wiedemann [Annalen der Physik 165, 497 (1853)] KN, P. Simon, and DL [Phys. Rev. B 92, 134425 (2015)] Fermion Boson WF law (Low temp.) 𝐿22 + 𝑂(𝜀 𝐹 −2 ) 𝐿11 ≡ 𝐾 𝜎 = 𝜋2 3 𝑘 𝐵 𝑒 2 𝑇 (Free electron at low temp.) 𝐿22 − 𝐿21 𝐿12 /𝐿11 𝐿11 ≡ 𝐾 𝐺 = 𝑘 𝐵 𝑔𝜇 𝐵 2 𝑇 [Low temp.: ℏ/(2𝜏) ≪ 𝑘 𝐵 𝑇 ≪ 𝑔𝜇 𝐵 𝐵] Lorenz number ℒ ≡ 𝜋2 3 𝑘 𝐵 𝒆 2 ℒm ≡ 𝑘 𝐵 𝒈𝝁 𝑩 2 Seebeck 𝑆 & Peltier Π 𝑆 ≡ 𝐿12 /𝐿11 , 𝛱 ≡ 𝐿21 /𝐿11 𝑆 = 𝐵/𝑇, 𝛱 = 𝐵 [Low temp.: ℏ/(2𝜏) ≪ 𝑘 𝐵 𝑇 ≪ 𝑔𝜇 𝐵 𝐵]  Universal Onsager relation 𝐿21 = 𝑇𝐿12 𝐿21 = 𝑇𝐿12 Thomson relation 𝛱 = 𝑇𝑆 𝛱 = 𝑇𝑆 Thermo-electric & –magnetic Effects
  • 23. CONCLUSION Ratio of 𝐿𝑖𝑗 : 𝐾/𝐺, 𝑆, 𝛱  Universal thermomagnetic properties (i.e., Not depend on materials)  Each Onsager coefficient 𝐿𝑖𝑗: Depend on materials
  • 24. SUMMARY 𝐾 𝐺 = 𝑘 𝐵 𝑔𝜇 𝐵 2 𝑇 ∝ 𝑇 𝐾 : Thermal magnon conductance, 𝐺: Magnetic magnon conductance Wiedemann-Franz Law for Magnon  Fundamental thermomagnetic relation of magnon transport in FI  Ratio of 𝐿𝑖𝑗: 𝐾/𝐺, 𝑆, 𝛱  Universal thermomagnetic properties Low temp.: ℏ/(2𝜏) ≪ 𝑘 𝐵 𝑇 ≪ 𝑔𝜇 𝐵 𝐵 𝑘B𝜇B `WF’ Magnet: 𝐺 Heat: 𝐾 Magnon (Boson) Electron (Fermion) `Universal’ Based on [Phys. Rev. B 92, 134425 (2015)] by KN, P. Simon, and D. Loss