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Active graphene metasurfaces for
optoelectronic applications
Nima Dabidian
Gennady Shvets group
University of Texas at Austin
1
Switching of Mid-IR light
Interferometric measurement of
phase modulation
High collection-efficiency
photo-detector
Sub-diffraction low threshold
nano-lasers
2
The goal:
• Ultra-fast devices for modulation of light intensity, phase ,
polarization state
• Ultra-fast detection of light intensity. Polarization state.
• Thin device
• Efficient
• Active material: mechanical tunability vs electrical
3
Mid-infrared optical properties of graphene
• Broadband response
• Small losses
𝜎 𝜔 = 𝜎𝑟 𝜔 + 𝑖 𝜎𝑖 𝜔
𝜎𝑟 ∶ Resistive
𝜎𝑖 : Inductive 𝝈𝒊/𝝈𝒓
S. H. Mousavi, e al, Nano Lett. 2013,
13,1111-1117 4
How to switch light
• A mode with narrow linewidth
(high quality factor)
• Large spectral shift (large field
enhancement)
• Zero reflectivity at the minimum
5
Double-Fano plasmonic metasurface
6
Enhanced near-fields due to second Fano
Monopole mode Dipole mode
7
Graphene interacts with tangential fields only
8
Graphene optical conductivity
𝜎 𝜔 = 𝜎𝑟 𝜔 + 𝜎𝑖 𝜔 𝜎0 =
𝑒2
4ℏ
9
Large modulation depth
Relative reflectivity:
Modulation depth: 80 %
Gap=70nm
Increasing doping
10
Higher modulation depth: 90 %
Gap=100nm
Dipole : ∆𝜔 𝑑 Γ𝑑 ≈ 80%
Monopole: ∆𝜔 𝑚 Γ 𝑚 ≈ 23 %
11
Triple-Lorenzian fit gives spectral position and life
time of the resonances
𝑟(𝜔)
2
fitted to
Exp. Reflectivity
12
QF enhancement near the phonon resonance
QF:
13
QF enhancement near the phonon resonance
𝜀 𝑒𝑓𝑓 =
𝜕𝜀 𝑟𝑒
𝜕𝜔
𝜔 + 𝜀 𝑟𝑒
14
Optimizing the optical response
of the resonances
𝜀 𝑒𝑓𝑓 =
𝜕𝜀 𝑟𝑒
𝜕𝜔
𝜔 + 𝜀 𝑟𝑒
15
Collisional time (𝝉) derivation from
the optical conductivity
Electrical transport measurement
𝜎 ∶ 𝐸𝑙𝑒𝑐𝑡𝑟𝑖𝑐𝑎𝑙 𝑐𝑜𝑛𝑑𝑢𝑐𝑡𝑖𝑣𝑖𝑡𝑦
𝜏 = 18 𝑓𝑠 (293 𝑐𝑚−1)
𝜏 = 14 𝑓𝑠
16
Interferometric measurement
of phase modulation
• Conventional phase modulator : bulk
• Metasurfaces cause abrupt phase shift
• Applications in
-Phased array antennas : beam steering
-Holograms
-Tunable lenses
-Tunable retarders
17
The experimental setup
Laser
BS
Graphene metasurface
Detector
𝐴𝑠𝑖𝑛(𝜔𝑡 + Φ1 𝑥 + Φ1 0 )
𝐵(𝑣)𝑠𝑖𝑛(𝜔𝑡 + Φ2(𝑉))
𝐶(𝑥, 𝑣, 𝑡)
Type equation here.
𝑥
𝑃1
18
𝑃2
Mirror on a
motorized stage
Beam
splitter
Mirror 1
Mirror 2
polarizer
lens
QCL
MCT
detector
pinhole1
pinhole2
19
Interference
• 𝐶 𝑡 = 𝐴𝑠𝑖𝑛 𝜔𝑡 + Φ1 𝑥 + Φ1 0 + 𝐵𝑠𝑖𝑛 𝜔𝑡 + Φ2 𝑉
• 𝐶(𝑥, 𝑉) 2
=
𝐴 2
2
+
𝐵 2
2
+ 𝐴𝐵𝑐𝑜𝑠(Φ1 𝑥 -Φ2 𝑉 + Φ1 0 )
𝑥: Mirror position
𝑉: 𝐺𝑟𝑎𝑝ℎ𝑒𝑛𝑒 𝑣𝑜𝑙𝑡𝑎𝑔𝑒
𝐶 𝑥, 𝑉 2 = a(v)cos 𝑏𝑥 + 𝑐(𝑣) + 𝑑(v)
intensity measurement (dots) fitted
to the function:
𝐶(𝑥,𝑉)2
𝑐(𝑣) = Φ1 0 − Φ2 𝑉
b= Φ1 𝑥
20
a(v) = AB(v),
d(v) =
A 2
2
+
B(v) 2
2
Phase change derivation
Step size of closed
loop actuator=63.5 nmΔΦ = Φ 𝑉1 − Φ 𝑉 = 0
= 𝑐(𝑉1) -c(0)
𝑉 = 0
𝑉 = 𝑉1
𝑉 = 0
𝑉 = 0
𝑏 𝑎𝑣𝑒𝑟𝑎𝑔𝑒 ≅ (𝑏1+𝑏2)/2
21
𝑓𝑖𝑡 𝑡𝑜 𝑐𝑜𝑠(𝑏 𝑎𝑣𝑒𝑟𝑎𝑔𝑒 𝑥 + 𝑐)
𝐼 𝑛𝑜𝑟𝑚 𝑥, 𝑣 =
C x,v 2−d(v)
a(v)
=
Fitted curves
Y-Pol X-Pol
23
Phase shift at 𝝀 = 𝟕. 𝟔𝟗𝝁𝒎
24
Comparison between Sim. & Exp.
25
Application example: Tunable retarder
𝐸𝑖𝑛𝑐 = 45°
26
Phase shift at 𝝀 = 𝟕. 𝟔𝟗𝝁𝒎
27
Application in ultra-fast motion detection
28
cos c v + b 𝑎𝑣𝑒x , Fitting parameter : x
Conclusion
• Dynamic modulation of amplitude, phase , polarization state of
Mid-IR light is made possible by integration of graphene to
Fano-resonance plasmonic metasurfaces
• Electrically connected metasurface provide the opportunities
for independent gating across metasurface and could be
potentially used in holographic application.
29
Acknowledgements
Collaborators:
Prof. Rod Ruoff (UT)
Iskandar Khomanov
A. Khanikaev,
Kaya Tatar,
Simeon Trendafilov,
S. Hossein Mousavi,
Carl Magnuson,
30
Thank you !
31

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My works slideshare hl

  • 1. Active graphene metasurfaces for optoelectronic applications Nima Dabidian Gennady Shvets group University of Texas at Austin 1
  • 2. Switching of Mid-IR light Interferometric measurement of phase modulation High collection-efficiency photo-detector Sub-diffraction low threshold nano-lasers 2
  • 3. The goal: • Ultra-fast devices for modulation of light intensity, phase , polarization state • Ultra-fast detection of light intensity. Polarization state. • Thin device • Efficient • Active material: mechanical tunability vs electrical 3
  • 4. Mid-infrared optical properties of graphene • Broadband response • Small losses 𝜎 𝜔 = 𝜎𝑟 𝜔 + 𝑖 𝜎𝑖 𝜔 𝜎𝑟 ∶ Resistive 𝜎𝑖 : Inductive 𝝈𝒊/𝝈𝒓 S. H. Mousavi, e al, Nano Lett. 2013, 13,1111-1117 4
  • 5. How to switch light • A mode with narrow linewidth (high quality factor) • Large spectral shift (large field enhancement) • Zero reflectivity at the minimum 5
  • 7. Enhanced near-fields due to second Fano Monopole mode Dipole mode 7
  • 8. Graphene interacts with tangential fields only 8
  • 9. Graphene optical conductivity 𝜎 𝜔 = 𝜎𝑟 𝜔 + 𝜎𝑖 𝜔 𝜎0 = 𝑒2 4ℏ 9
  • 10. Large modulation depth Relative reflectivity: Modulation depth: 80 % Gap=70nm Increasing doping 10
  • 11. Higher modulation depth: 90 % Gap=100nm Dipole : ∆𝜔 𝑑 Γ𝑑 ≈ 80% Monopole: ∆𝜔 𝑚 Γ 𝑚 ≈ 23 % 11
  • 12. Triple-Lorenzian fit gives spectral position and life time of the resonances 𝑟(𝜔) 2 fitted to Exp. Reflectivity 12
  • 13. QF enhancement near the phonon resonance QF: 13
  • 14. QF enhancement near the phonon resonance 𝜀 𝑒𝑓𝑓 = 𝜕𝜀 𝑟𝑒 𝜕𝜔 𝜔 + 𝜀 𝑟𝑒 14
  • 15. Optimizing the optical response of the resonances 𝜀 𝑒𝑓𝑓 = 𝜕𝜀 𝑟𝑒 𝜕𝜔 𝜔 + 𝜀 𝑟𝑒 15
  • 16. Collisional time (𝝉) derivation from the optical conductivity Electrical transport measurement 𝜎 ∶ 𝐸𝑙𝑒𝑐𝑡𝑟𝑖𝑐𝑎𝑙 𝑐𝑜𝑛𝑑𝑢𝑐𝑡𝑖𝑣𝑖𝑡𝑦 𝜏 = 18 𝑓𝑠 (293 𝑐𝑚−1) 𝜏 = 14 𝑓𝑠 16
  • 17. Interferometric measurement of phase modulation • Conventional phase modulator : bulk • Metasurfaces cause abrupt phase shift • Applications in -Phased array antennas : beam steering -Holograms -Tunable lenses -Tunable retarders 17
  • 18. The experimental setup Laser BS Graphene metasurface Detector 𝐴𝑠𝑖𝑛(𝜔𝑡 + Φ1 𝑥 + Φ1 0 ) 𝐵(𝑣)𝑠𝑖𝑛(𝜔𝑡 + Φ2(𝑉)) 𝐶(𝑥, 𝑣, 𝑡) Type equation here. 𝑥 𝑃1 18 𝑃2 Mirror on a motorized stage
  • 20. Interference • 𝐶 𝑡 = 𝐴𝑠𝑖𝑛 𝜔𝑡 + Φ1 𝑥 + Φ1 0 + 𝐵𝑠𝑖𝑛 𝜔𝑡 + Φ2 𝑉 • 𝐶(𝑥, 𝑉) 2 = 𝐴 2 2 + 𝐵 2 2 + 𝐴𝐵𝑐𝑜𝑠(Φ1 𝑥 -Φ2 𝑉 + Φ1 0 ) 𝑥: Mirror position 𝑉: 𝐺𝑟𝑎𝑝ℎ𝑒𝑛𝑒 𝑣𝑜𝑙𝑡𝑎𝑔𝑒 𝐶 𝑥, 𝑉 2 = a(v)cos 𝑏𝑥 + 𝑐(𝑣) + 𝑑(v) intensity measurement (dots) fitted to the function: 𝐶(𝑥,𝑉)2 𝑐(𝑣) = Φ1 0 − Φ2 𝑉 b= Φ1 𝑥 20 a(v) = AB(v), d(v) = A 2 2 + B(v) 2 2
  • 21. Phase change derivation Step size of closed loop actuator=63.5 nmΔΦ = Φ 𝑉1 − Φ 𝑉 = 0 = 𝑐(𝑉1) -c(0) 𝑉 = 0 𝑉 = 𝑉1 𝑉 = 0 𝑉 = 0 𝑏 𝑎𝑣𝑒𝑟𝑎𝑔𝑒 ≅ (𝑏1+𝑏2)/2 21 𝑓𝑖𝑡 𝑡𝑜 𝑐𝑜𝑠(𝑏 𝑎𝑣𝑒𝑟𝑎𝑔𝑒 𝑥 + 𝑐) 𝐼 𝑛𝑜𝑟𝑚 𝑥, 𝑣 = C x,v 2−d(v) a(v) =
  • 24. Phase shift at 𝝀 = 𝟕. 𝟔𝟗𝝁𝒎 24
  • 26. Application example: Tunable retarder 𝐸𝑖𝑛𝑐 = 45° 26
  • 27. Phase shift at 𝝀 = 𝟕. 𝟔𝟗𝝁𝒎 27
  • 28. Application in ultra-fast motion detection 28 cos c v + b 𝑎𝑣𝑒x , Fitting parameter : x
  • 29. Conclusion • Dynamic modulation of amplitude, phase , polarization state of Mid-IR light is made possible by integration of graphene to Fano-resonance plasmonic metasurfaces • Electrically connected metasurface provide the opportunities for independent gating across metasurface and could be potentially used in holographic application. 29
  • 30. Acknowledgements Collaborators: Prof. Rod Ruoff (UT) Iskandar Khomanov A. Khanikaev, Kaya Tatar, Simeon Trendafilov, S. Hossein Mousavi, Carl Magnuson, 30