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Characterization of Aerosol Events using the Federated Data System, DataFed R.B. Husar and S.R. Falke  Washington University in St. Louis Presented at EPA – OAQPS Seminar Research Triangle Park, NC, November 1, 2005
Regional Haze Rule: Natural Aerosol ,[object Object],[object Object]
NAAMS:  National Ambient Air Monitoring Strategy  and NCore … coordinated multi-pollutant real-time monitoring network
Natural and Exceptional Event Rule (Making) ,[object Object],[object Object],[object Object]
Dust, Smoke and Exceptional Events Intercontinental Dust Smoke  Event July 4 2004 July 4 2003
Long-Term Monitoring: Fine Mass, SO4, K ,[object Object],[object Object],[object Object],[object Object],Sulfate Fine Mass Potassium
Evolution of Spatial Data Coverage: Fine Sulfate, 1998-2003 ,[object Object],[object Object],[object Object],1998 1999 2000 2003 2002 2001
AIRNOW PM25 -  ASOS RH- Corrected Bext  July 21, 2004 July 22, 2004 July 23, 2004 ARINOW PM25 ARINOW PM25 ARINOW PM25 ASOS RHBext ASOS RHBext ASOS RHBext
Quebec Smoke July 7, 2002 Satellite Optical Depth & Surface ASOS RHBext
Event Detection   Temporal Signal Decomposition ,[object Object],[object Object],EUS Daily Average 50%-ile, 30 day 50%-ile smoothing Deviation from %-ile Event : Deviation > x*percentile Median Seasonal Conc. Mean Seasonal Conc. Average Median ,[object Object]
Seasonal PM25 by Region ,[object Object],[object Object],[object Object]
Bext Distribution Function Albany  Sigma g =  3.75 Charlotte Sigma g = 1.56 Upper 20 percentile contribution: Notheast > 50% of dosage Southeast < 30% of dosage 1979
Application of Automatic Event Detection: A Trigger and Screening Tool ,[object Object],[object Object],[object Object]
Causes  of Temporal Variation by Region ,[object Object],[object Object],[object Object],[object Object],Northeast  exhibits the largest coeff. variation (56%); seasonal, noise and events each at 30% Southeast  is the least variable region (35%), with virtually no contribution from events Southwest, Northwest, S. Cal. and Great Lakes/Plains  show 40-50% coeff. variation mostly, due to seasonal and meteorological noise. Interestingly,  the noise is about 30% in all regions, while the events vary much more, 5-30%
‘Composition’ of Eastern US Events ,[object Object],[object Object],[object Object],[object Object],Based on VIEWS data
The largest EUS Regional PM Event: Nov 15, 2005
Early Satellite Detection of Manmade Haze, 1976  Regional Haze Low Visibility Hazy ‘Blobs’ Lyons W.A., Husar R.B.  Mon. Weather Rev.   1976 SMS GOES June 30 1975
SeaWiFS AOT – Summer 60 Percentile 1 km Resolution
Satellite Aerosol Optical Thickness Climatology SeaWiFS Satellite, Summer 2000 - 2003 20 Percentile 99 Percentile 90 Percentile 60 Percentile
Average and 98 Percentile Pattern SO4 PM2.5 Mass PM2.5 Mass OC  OC  SO4 A V E R A G E 98 Percentile
Estimation of Smoke Mass ,[object Object],[object Object],[object Object],[object Object],[object Object],[object Object]
Smoke Quantification using Chemical Data ,[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],[object Object]
Smoke Excess OC – EC Calibration of SmokeBiogenic Composition ,[object Object],[object Object],[object Object], PM25  EC  OC SmokeBiogenic:  EC/  OC  = 0.08  PM25/  OC  = 1.5 EC/OC Ratio
Soot OC–EC Calibration by Iteration ,[object Object],[object Object],[object Object],EC/OC Soot = 0.15 EC/OC Soot = 0.2 EC/OC Soot = 1 EC/OC Soot = 0.4 Negative SmokeBio – not Possible Maybe?? Maybe?? Too little soot,  too much smokebio SmokeBio OC Soot OC
Measured and Reconstructed PM25 Mass ,[object Object]
OCSB, OCSoot and PM25 Seasonal Pattern Average over 2000-2004 period PM25Mass OCSB SmokeBio OCSoot Day of Year Mexican Smoke Agricultural Smoke Urban Soot
OC SmokeBiogenic Spatial Pattern Dec Jan Feb Sep Oct Nov Mar Apr May Jun Jul Aug
Soot Spatial Pattern Dec Jan Feb Sep Oct Nov Mar Apr May Jun Jul Aug Jun Jul Aug
PM2.5 (blue) and SmokeBioMass (red)   Note: Smoke events are spikes superimposed on biogenic OC background Smoke Events Kansas Agric. Smoke
Example OC Smoke Events Note: Smoke events are spikes superimposed on biogenic OC background Smoke Events
GRSM Seasonal Pattern of Percentiles PM25 OC SO4 Soil Episodic Episodic OC in Fall dominates episodicity -  Smoke Organics?
Monthly Maps of Fire Pixels ,[object Object],[object Object],NOAA HMS – S. Falke Jan Feb Mar Apr Aug Jun Jul May Sep Oct Nov Dec Smoke Kansas Ag Smoke No Smoke
Summary ,[object Object],[object Object],[object Object],[object Object],[object Object],[object Object],[object Object]
FASTNET: Inter-RPO pilot project, through NESCAUM, 2004 Web-based data, tools for community use Built on DataFed infra-structure, NSF, NASA Project fate depends on sponsor, user evaluation
Some of the DataFed Tools ,[object Object],[object Object],[object Object],[object Object],Consoles:  Data from diverse sources are displayed to create a rich context for exploration and analysis CATT:  Combined Aerosol Trajectory Tool for the browsing backtrajectories for specified chemical conditions  Viewer:  General purpose spatio-temporal data browser and view editor applicable for all DataFed datasets
Conceptual Diagram of an Emissions Community XML GIS Estimation Methods RDBMS Geospatial One-Stop Transport Models Emissions Inventory Catalog Users & Projects Web  Tools/Services Emissions Inventories Data Data Catalogs Activity Data Spatial  Allocation Comparison  of Emissions  Methods Data Analysis Model  Development Wrappers Emissions Factors Surrogates Report Generation Mediators / Portal
North American Commission  for Environmental Cooperation   Web Application Report http:// www.cec.org /files/PDF/ POLLUTANTS/ PowerPlant_AirEmission_en.pdf http:// webapps.datafed.net/dvoy_services / datafed.aspx?page = PowerPlant_Emissions 2002 North American Powerplant Emissions
Spatial-temporal analysis of fire counts   http:// webapps.datafed.net/dvoy_services/datafed.aspx?page =Fire_Pixel_Count_AK   Large fires during the summer of 2004 in Central Alaska.  Spatially aggregated count of fire pixels over a 100km 2  area.  The size of each red square in the map is proportional to the number of fire pixels. The spatial aggregation allows the generation of a time series for each aggregated area.
BLM Area burned  - monthly average The acres burned in the BLM compiled fire history dataset are  spatially aggregated  on a 50km 2  grid and  temporally aggregated  to a monthly resolution.  Circles are proportional to the acres burned at a location for a particular year and month.  Time series plot shows the monthly total number of acres burned at a particular 50km2 area.  http:// webapps.datafed.net/dvoy_services/datafed.aspx?page = BLM_AcresBurned
Aggregation Tools Fire Pixels June 16-23, 2004 Spatially Aggregated Monthly Sum Spatially Aggregated
Spatial-temporal Comparison of fire pixels   http://www.datafed.net/WebApps/MiscApps/ModisGoes/FireLocationComparison.htm   A  red  shaded  square indicates a  short distance  separating the MODIS and GOES pixels while a  blue  shaded  square indicates the nearest neighbor between the datasets were  far apart .  A  red  outlined   square indicates the nearest neighbor was detected on the  same day  while a  blue  outlined  square indicates a  longer time separation .  Gray shaded and/or outlined  squares indicate that a nearest neighbor was not found between the two datasets given the search parameters (in this example case, 100 km and 2 days).
Standards Based Data Sharing Open Geospatial Specifications (OGC) for web mapping Web Map Service (images) Web Feature Service (point/vector data) Web Coverage Service (gridded data) Geospatial One-Stop – The National Map DataFed-OGC Description:   http:// www.datafed.net/DataLinks/OGC/OGC.htm http://webapps.datafed.net/dvoy_services/ogc_domain_fire.wsfl?SERVICE=WMS&VERSION=1.1.1&REQUEST=GetCapabilities   DataFed OGC WMS for fire data:
Seasonality of OC Percentiles ,[object Object],Great Smoky Mtn: Episodic OC in  the Fall season Chattanooga:: Elevated and Persistent OC
 
Field burning particulate pollution & asthma - Shorts ,[object Object],[object Object],[object Object],[object Object]
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0507 Event Analysis 051101 Event Seminar2

  • 1. Characterization of Aerosol Events using the Federated Data System, DataFed R.B. Husar and S.R. Falke Washington University in St. Louis Presented at EPA – OAQPS Seminar Research Triangle Park, NC, November 1, 2005
  • 2.
  • 3. NAAMS: National Ambient Air Monitoring Strategy and NCore … coordinated multi-pollutant real-time monitoring network
  • 4.
  • 5. Dust, Smoke and Exceptional Events Intercontinental Dust Smoke Event July 4 2004 July 4 2003
  • 6.
  • 7.
  • 8. AIRNOW PM25 - ASOS RH- Corrected Bext July 21, 2004 July 22, 2004 July 23, 2004 ARINOW PM25 ARINOW PM25 ARINOW PM25 ASOS RHBext ASOS RHBext ASOS RHBext
  • 9. Quebec Smoke July 7, 2002 Satellite Optical Depth & Surface ASOS RHBext
  • 10.
  • 11.
  • 12. Bext Distribution Function Albany Sigma g = 3.75 Charlotte Sigma g = 1.56 Upper 20 percentile contribution: Notheast > 50% of dosage Southeast < 30% of dosage 1979
  • 13.
  • 14.
  • 15.
  • 16. The largest EUS Regional PM Event: Nov 15, 2005
  • 17. Early Satellite Detection of Manmade Haze, 1976 Regional Haze Low Visibility Hazy ‘Blobs’ Lyons W.A., Husar R.B. Mon. Weather Rev. 1976 SMS GOES June 30 1975
  • 18. SeaWiFS AOT – Summer 60 Percentile 1 km Resolution
  • 19. Satellite Aerosol Optical Thickness Climatology SeaWiFS Satellite, Summer 2000 - 2003 20 Percentile 99 Percentile 90 Percentile 60 Percentile
  • 20. Average and 98 Percentile Pattern SO4 PM2.5 Mass PM2.5 Mass OC OC SO4 A V E R A G E 98 Percentile
  • 21.
  • 22.
  • 23.
  • 24.
  • 25.
  • 26. OCSB, OCSoot and PM25 Seasonal Pattern Average over 2000-2004 period PM25Mass OCSB SmokeBio OCSoot Day of Year Mexican Smoke Agricultural Smoke Urban Soot
  • 27. OC SmokeBiogenic Spatial Pattern Dec Jan Feb Sep Oct Nov Mar Apr May Jun Jul Aug
  • 28. Soot Spatial Pattern Dec Jan Feb Sep Oct Nov Mar Apr May Jun Jul Aug Jun Jul Aug
  • 29. PM2.5 (blue) and SmokeBioMass (red) Note: Smoke events are spikes superimposed on biogenic OC background Smoke Events Kansas Agric. Smoke
  • 30. Example OC Smoke Events Note: Smoke events are spikes superimposed on biogenic OC background Smoke Events
  • 31. GRSM Seasonal Pattern of Percentiles PM25 OC SO4 Soil Episodic Episodic OC in Fall dominates episodicity - Smoke Organics?
  • 32.
  • 33.
  • 34. FASTNET: Inter-RPO pilot project, through NESCAUM, 2004 Web-based data, tools for community use Built on DataFed infra-structure, NSF, NASA Project fate depends on sponsor, user evaluation
  • 35.
  • 36. Conceptual Diagram of an Emissions Community XML GIS Estimation Methods RDBMS Geospatial One-Stop Transport Models Emissions Inventory Catalog Users & Projects Web Tools/Services Emissions Inventories Data Data Catalogs Activity Data Spatial Allocation Comparison of Emissions Methods Data Analysis Model Development Wrappers Emissions Factors Surrogates Report Generation Mediators / Portal
  • 37. North American Commission for Environmental Cooperation Web Application Report http:// www.cec.org /files/PDF/ POLLUTANTS/ PowerPlant_AirEmission_en.pdf http:// webapps.datafed.net/dvoy_services / datafed.aspx?page = PowerPlant_Emissions 2002 North American Powerplant Emissions
  • 38. Spatial-temporal analysis of fire counts http:// webapps.datafed.net/dvoy_services/datafed.aspx?page =Fire_Pixel_Count_AK Large fires during the summer of 2004 in Central Alaska. Spatially aggregated count of fire pixels over a 100km 2 area. The size of each red square in the map is proportional to the number of fire pixels. The spatial aggregation allows the generation of a time series for each aggregated area.
  • 39. BLM Area burned - monthly average The acres burned in the BLM compiled fire history dataset are spatially aggregated on a 50km 2 grid and temporally aggregated to a monthly resolution. Circles are proportional to the acres burned at a location for a particular year and month. Time series plot shows the monthly total number of acres burned at a particular 50km2 area. http:// webapps.datafed.net/dvoy_services/datafed.aspx?page = BLM_AcresBurned
  • 40. Aggregation Tools Fire Pixels June 16-23, 2004 Spatially Aggregated Monthly Sum Spatially Aggregated
  • 41. Spatial-temporal Comparison of fire pixels http://www.datafed.net/WebApps/MiscApps/ModisGoes/FireLocationComparison.htm A red shaded square indicates a short distance separating the MODIS and GOES pixels while a blue shaded square indicates the nearest neighbor between the datasets were far apart . A red outlined square indicates the nearest neighbor was detected on the same day while a blue outlined square indicates a longer time separation . Gray shaded and/or outlined squares indicate that a nearest neighbor was not found between the two datasets given the search parameters (in this example case, 100 km and 2 days).
  • 42. Standards Based Data Sharing Open Geospatial Specifications (OGC) for web mapping Web Map Service (images) Web Feature Service (point/vector data) Web Coverage Service (gridded data) Geospatial One-Stop – The National Map DataFed-OGC Description: http:// www.datafed.net/DataLinks/OGC/OGC.htm http://webapps.datafed.net/dvoy_services/ogc_domain_fire.wsfl?SERVICE=WMS&VERSION=1.1.1&REQUEST=GetCapabilities DataFed OGC WMS for fire data:
  • 43.
  • 44.  
  • 45.